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Dataset Open Access

Phase-resolved Higgs response in superconducting cuprates

Chu, Hao; Kim, Min-Jae; Katsumi, Kota; Kovalev, Sergey; Dawson, Robert David; Schwarz, Lukas; Yoshikawa, Naotaka; Kim, Gideok; Putzky, Daniel; Li, Zhi Zhong; Raffy, Hélène; Germanskiy, Semen; Deinert, Jan-Christoph; Awari, Nilesh; Ilyakov, Igor; Green, Bertram Windisch; Chen, Min; Bawatna, Mohammed; Christiani, Georg; Logvenov, Gennady; Gallais, Yann; Boris, Alexander V.; Keimer, Bernhard; Schnyder, Andreas; Manske, Dirk; Gensch, Michael; Wang, Zhe; Shimano, Ryo; Kaiser, Stefan

In high energy physics, the Higgs field couples to gauge bosons and fermions and gives mass to their elementary excitations. Experimentally, such couplings can be verified from the decay product of the Higgs boson, the scalar (amplitude) excitation of the Higgs field. In superconductors, Cooper pairs bear a certain analogy to the Higgs field. Coulomb interactions between the Cooper pairs give mass to the electromagnetic field, which leads to the Meissner effect. Additional coupling with other types of interactions or collective modes is foreseeable, and even highly probable for high-Tc superconductors, where multiple degrees of freedom are intertwined. The superconducting Higgs mode may reveal such couplings spectroscopically and uncover interactions directly relevant to Cooper pairing. To this end, we investigate the Higgs mode of several cuprate thin films using phase-resolved terahertz third harmonic generation (THG) to. In addition to the heavily damped Higgs mode itself, we observe a universal jump in the phase of the driven Higgs oscillation as well as a non-vanishing THG above Tc. These findings indicate coupling of the Higgs mode to other collective modes and a nonzero pairing amplitude above Tc. Our study demonstrates a new approach for investigating unconventional superconductivity. We foresee a fruitful future for phase-resolved spectroscopy in various superconducting systems.

Files (2.0 TB)
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14.7 GB Download
194_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_100K_15.06.2018_2340_36.rar
md5:26a5c59b804167c3049d141830a0c51a
14.6 GB Download
195_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_105K_15.06.2018_2349_09.rar
md5:7577fd348b7b39a2374ace542a880c63
14.6 GB Download
196_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_110K_15.06.2018_2357_18.rar
md5:d0c36e416e68e9f2b8aa27df0b550d63
7.5 GB Download
197_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_123K_16.06.2018_0042_45.rar
md5:0eeca14b87738ad657223de2fe42565f
14.5 GB Download
198_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_135K_16.06.2018_0055_11.rar
md5:611123a9d72179bc78ed64089b56c17a
4.6 GB Download
199_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_125K_16.06.2018_0100_17.rar
md5:fb3036d6ff405283297ca33ebfbd0c9c
14.5 GB Download
200_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_135K_16.06.2018_0112_26.rar
md5:2d1ec0c044323cbf42e53f8a346fbb04
14.5 GB Download
203_0p7THz_DyBCO_THG_HWP_126_P2_49_P3_180_P3p5_227_54p8K_16.06.2018_0204_58.rar
md5:b99faaf0956d9ed9c05f4ef36066f174
14.5 GB Download
204_0p7THz_DyBCO_THG_HWP_130_P2_59_P3_190_P3p5_227_54p7K_16.06.2018_0217_42.rar
md5:76bec8dc0c51fcbcd4e342006195bfc2
14.5 GB Download
205_0p7THz_DyBCO_THG_HWP_134_P2_65_P3_196_P3p5_227_54p7K_16.06.2018_0224_12.rar
md5:b535c0895f4a8daa7701a2fd50c447ac
14.5 GB Download
206_0p7THz_DyBCO_THG_HWP_137_P2_71_P3_202_P3p5_227_54p7K_16.06.2018_0230_38.rar
md5:d205668af9ee26a3b6b461465975ff56
14.5 GB Download
207_0p7THz_DyBCO_THG_HWP_140_P2_78_P3_209_P3p5_227_54p7K_16.06.2018_0237_02.rar
md5:20305b7f46b32fd6fb458ffc9c921769
14.5 GB Download
208_0p7THz_DyBCO_THG_HWP_142_P2_82_P3_213_P3p5_227_54p7K_16.06.2018_0243_51.rar
md5:c7f1cfe9b7f59ed6e1a3f4a958718403
14.5 GB Download
209_0p7THz_DyBCO_THG_HWP_147_P2_94_P3_225_P3p5_227_54p7K_16.06.2018_0250_30.rar
md5:eafe1b5dc7fda14adf640ffea471fae9
14.6 GB Download
210_0p7THz_DyBCO_THG_HWP_152_P2_106_P3_237_P3p5_227_54p7K_16.06.2018_0258_44.rar
md5:03940c98beb184be939284d19eaceb3d
14.5 GB Download
211_0p7THz_DyBCO_THG_HWP_154_P2_110_P3_241_P3p5_227_54p7K_16.06.2018_0305_20.rar
md5:62d7300277ede5852cdfc7f87a56351f
14.6 GB Download
212_0p7THz_DyBCO_THG_HWP_157_P2_117_P3_248_P3p5_227_54p7K_16.06.2018_0312_22.rar
md5:f912098027faaa22d6fbaca4d5d72f73
14.5 GB Download
213_0p7THz_DyBCO_THG_HWP_160_P2_123_P3_254_P3p5_227_54p7K_16.06.2018_0321_27.rar
md5:9832870133f82a2d7dd0fedaa678f1ed
14.4 GB Download
214_0p7THz_DyBCO_THG_HWP_160_P2_123_P3_254_P3p5_227_54p7K_16.06.2018_0411_20.rar
md5:be1f034762c30e2ce3d2abb4e967c3a1
14.6 GB Download
215_0p7THz_DyBCO_THG_HWP_161_P2_129_P3_260_P3p5_227_54p7K_16.06.2018_0417_37.rar
md5:bc69e293644548059a01dfbb5c5ee0e7
14.7 GB Download
216_0p7THz_DyBCO_THG_HWP_161_P2_137_P3_270_P3p5_227_54p7K_16.06.2018_0423_49.rar
md5:078827614b21f0c4402e23acaf7081ec
14.7 GB Download
217_0p7THz_DyBCO_THG_HWP_161_P2_137_P3_270_P3p5_227_54p7K_16.06.2018_0433_51.rar
md5:f90f15c6dd36933626fdb220ea603899
14.8 GB Download
218_0p7THz_DyBCO_THG_HWP_137_P2_71_P3_202_P3p5_249_54p7K_16.06.2018_0444_37.rar
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14.7 GB Download
219_0p7THz_DyBCO_THG_HWP_137_P2_71_P3_112_P3p5_249_54p7K_16.06.2018_0451_27.rar
md5:c95a795c8b6169085ae209859a80353f
14.8 GB Download
Data analysis.zip
md5:d41d8cd98f00b204e9800998ecf8427e
1.7 MB Download
Labbook_Dec. 2018 Higgs.zip
md5:10206f47ac188ea12011b5aff7ade675
72.2 MB Download
Labbook_June2018 Higgs.zip
md5:0bead7dd45ad6261a345ecf16ded6147
40.3 MB Download
README_rodare.txt
md5:98a62a172e5cb650ab5f787fdce4d2e6
2.5 kB Download
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