Dataset Open Access

Phase-resolved Higgs response in superconducting cuprates

Chu, Hao; Kim, Min-Jae; Katsumi, Kota; Kovalev, Sergey; Dawson, Robert David; Schwarz, Lukas; Yoshikawa, Naotaka; Kim, Gideok; Putzky, Daniel; Li, Zhi Zhong; Raffy, Hélène; Germanskiy, Semen; Deinert, Jan-Christoph; Awari, Nilesh; Ilyakov, Igor; Green, Bertram Windisch; Chen, Min; Bawatna, Mohammed; Christiani, Georg; Logvenov, Gennady; Gallais, Yann; Boris, Alexander V.; Keimer, Bernhard; Schnyder, Andreas; Manske, Dirk; Gensch, Michael; Wang, Zhe; Shimano, Ryo; Kaiser, Stefan

In high energy physics, the Higgs field couples to gauge bosons and fermions and gives mass to their elementary excitations. Experimentally, such couplings can be verified from the decay product of the Higgs boson, the scalar (amplitude) excitation of the Higgs field. In superconductors, Cooper pairs bear a certain analogy to the Higgs field. Coulomb interactions between the Cooper pairs give mass to the electromagnetic field, which leads to the Meissner effect. Additional coupling with other types of interactions or collective modes is foreseeable, and even highly probable for high-Tc superconductors, where multiple degrees of freedom are intertwined. The superconducting Higgs mode may reveal such couplings spectroscopically and uncover interactions directly relevant to Cooper pairing. To this end, we investigate the Higgs mode of several cuprate thin films using phase-resolved terahertz third harmonic generation (THG) to. In addition to the heavily damped Higgs mode itself, we observe a universal jump in the phase of the driven Higgs oscillation as well as a non-vanishing THG above Tc. These findings indicate coupling of the Higgs mode to other collective modes and a nonzero pairing amplitude above Tc. Our study demonstrates a new approach for investigating unconventional superconductivity. We foresee a fruitful future for phase-resolved spectroscopy in various superconducting systems.

Files (2.0 TB)
Name Size
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14.7 GB Download
194_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_100K_15.06.2018_2340_36.rar
md5:26a5c59b804167c3049d141830a0c51a
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195_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_105K_15.06.2018_2349_09.rar
md5:7577fd348b7b39a2374ace542a880c63
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196_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_110K_15.06.2018_2357_18.rar
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197_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_123K_16.06.2018_0042_45.rar
md5:0eeca14b87738ad657223de2fe42565f
14.5 GB Download
198_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_135K_16.06.2018_0055_11.rar
md5:611123a9d72179bc78ed64089b56c17a
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199_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_125K_16.06.2018_0100_17.rar
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200_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_135K_16.06.2018_0112_26.rar
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203_0p7THz_DyBCO_THG_HWP_126_P2_49_P3_180_P3p5_227_54p8K_16.06.2018_0204_58.rar
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204_0p7THz_DyBCO_THG_HWP_130_P2_59_P3_190_P3p5_227_54p7K_16.06.2018_0217_42.rar
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205_0p7THz_DyBCO_THG_HWP_134_P2_65_P3_196_P3p5_227_54p7K_16.06.2018_0224_12.rar
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206_0p7THz_DyBCO_THG_HWP_137_P2_71_P3_202_P3p5_227_54p7K_16.06.2018_0230_38.rar
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207_0p7THz_DyBCO_THG_HWP_140_P2_78_P3_209_P3p5_227_54p7K_16.06.2018_0237_02.rar
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208_0p7THz_DyBCO_THG_HWP_142_P2_82_P3_213_P3p5_227_54p7K_16.06.2018_0243_51.rar
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209_0p7THz_DyBCO_THG_HWP_147_P2_94_P3_225_P3p5_227_54p7K_16.06.2018_0250_30.rar
md5:eafe1b5dc7fda14adf640ffea471fae9
14.6 GB Download
210_0p7THz_DyBCO_THG_HWP_152_P2_106_P3_237_P3p5_227_54p7K_16.06.2018_0258_44.rar
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211_0p7THz_DyBCO_THG_HWP_154_P2_110_P3_241_P3p5_227_54p7K_16.06.2018_0305_20.rar
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212_0p7THz_DyBCO_THG_HWP_157_P2_117_P3_248_P3p5_227_54p7K_16.06.2018_0312_22.rar
md5:f912098027faaa22d6fbaca4d5d72f73
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213_0p7THz_DyBCO_THG_HWP_160_P2_123_P3_254_P3p5_227_54p7K_16.06.2018_0321_27.rar
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214_0p7THz_DyBCO_THG_HWP_160_P2_123_P3_254_P3p5_227_54p7K_16.06.2018_0411_20.rar
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215_0p7THz_DyBCO_THG_HWP_161_P2_129_P3_260_P3p5_227_54p7K_16.06.2018_0417_37.rar
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216_0p7THz_DyBCO_THG_HWP_161_P2_137_P3_270_P3p5_227_54p7K_16.06.2018_0423_49.rar
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217_0p7THz_DyBCO_THG_HWP_161_P2_137_P3_270_P3p5_227_54p7K_16.06.2018_0433_51.rar
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218_0p7THz_DyBCO_THG_HWP_137_P2_71_P3_202_P3p5_249_54p7K_16.06.2018_0444_37.rar
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219_0p7THz_DyBCO_THG_HWP_137_P2_71_P3_112_P3p5_249_54p7K_16.06.2018_0451_27.rar
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Data analysis.zip
md5:d41d8cd98f00b204e9800998ecf8427e
1.7 MB Download
Labbook_Dec. 2018 Higgs.zip
md5:10206f47ac188ea12011b5aff7ade675
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Labbook_June2018 Higgs.zip
md5:0bead7dd45ad6261a345ecf16ded6147
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README_rodare.txt
md5:98a62a172e5cb650ab5f787fdce4d2e6
2.5 kB Download
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