Dataset Open Access

Phase-resolved Higgs response in superconducting cuprates

Chu, Hao; Kim, Min-Jae; Katsumi, Kota; Kovalev, Sergey; Dawson, Robert David; Schwarz, Lukas; Yoshikawa, Naotaka; Kim, Gideok; Putzky, Daniel; Li, Zhi Zhong; Raffy, Hélène; Germanskiy, Semen; Deinert, Jan-Christoph; Awari, Nilesh; Ilyakov, Igor; Green, Bertram Windisch; Chen, Min; Bawatna, Mohammed; Christiani, Georg; Logvenov, Gennady; Gallais, Yann; Boris, Alexander V.; Keimer, Bernhard; Schnyder, Andreas; Manske, Dirk; Gensch, Michael; Wang, Zhe; Shimano, Ryo; Kaiser, Stefan

In high energy physics, the Higgs field couples to gauge bosons and fermions and gives mass to their elementary excitations. Experimentally, such couplings can be verified from the decay product of the Higgs boson, the scalar (amplitude) excitation of the Higgs field. In superconductors, Cooper pairs bear a certain analogy to the Higgs field. Coulomb interactions between the Cooper pairs give mass to the electromagnetic field, which leads to the Meissner effect. Additional coupling with other types of interactions or collective modes is foreseeable, and even highly probable for high-Tc superconductors, where multiple degrees of freedom are intertwined. The superconducting Higgs mode may reveal such couplings spectroscopically and uncover interactions directly relevant to Cooper pairing. To this end, we investigate the Higgs mode of several cuprate thin films using phase-resolved terahertz third harmonic generation (THG) to. In addition to the heavily damped Higgs mode itself, we observe a universal jump in the phase of the driven Higgs oscillation as well as a non-vanishing THG above Tc. These findings indicate coupling of the Higgs mode to other collective modes and a nonzero pairing amplitude above Tc. Our study demonstrates a new approach for investigating unconventional superconductivity. We foresee a fruitful future for phase-resolved spectroscopy in various superconducting systems.

Files (2.7 TB)
Name Size
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20.3 GB Download
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20.3 GB Download
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20.3 GB Download
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20.3 GB Download
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20.3 GB Download
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20.3 GB Download
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20.3 GB Download
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20.3 GB Download
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20.2 GB Download
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19.9 GB Download
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19.5 GB Download
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md5:58fd560131cea8e91b8ac85afb4ff918
19.7 GB Download
189_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_75K_15.06.2018_2249_25.zip
md5:fa212e7e4a0353b4f4044edfa4782079
19.7 GB Download
190_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_80K_15.06.2018_2301_03.zip
md5:cba16a39075c4f849b357e6688aa8656
19.6 GB Download
191_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_85K_15.06.2018_2310_21.zip
md5:05b10a55affcdf1dfffd5fbbcfd64aa2
19.7 GB Download
192_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_90K_15.06.2018_2319_36.zip
md5:625f7446ea63be966f4dc53b360fd8d0
19.7 GB Download
193_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_95K_15.06.2018_2328_10.zip
md5:a66b49326e940f4cd533af77b1fa6bd5
19.7 GB Download
194_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_100K_15.06.2018_2340_36.zip
md5:a57744c0d522543efa17be2d899bf52b
19.7 GB Download
195_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_105K_15.06.2018_2349_09.zip
md5:12924baf7bce11e38bcd1e5a214af7b2
19.7 GB Download
196_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_110K_15.06.2018_2357_18.zip
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10.0 GB Download
197_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_123K_16.06.2018_0042_45.zip
md5:6834bcddb7a430919e0183ef2ea2d67b
19.6 GB Download
198_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_135K_16.06.2018_0055_11.zip
md5:6e464c30d5f927756b1fb63c747c0c75
6.3 GB Download
199_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_125K_16.06.2018_0100_17.zip
md5:3f234317859b3e2543f3807092a2abba
19.7 GB Download
200_0p7THz_DyBCO_THG_P1_157_P2_49_P3_180_135K_16.06.2018_0112_26.zip
md5:31ebea3ab867f336c75e9487193263ef
19.7 GB Download
201_0p7THz_DyBCO_THG_HWP_126_P2_49_P3_180_P3p5_227_55K_16.06.2018_0149_33.zip
md5:fc3a0fe445621a0c2be9efdad25015de
19.7 GB Download
202_0p7THz_DyBCO_THG_HWP_130_P2_59_P3_190_P3p5_227_55K_16.06.2018_0156_31.zip
md5:274cb0ee392cf2d6e58bbdd6da6eebe1
19.7 GB Download
203_0p7THz_DyBCO_THG_HWP_126_P2_49_P3_180_P3p5_227_54p8K_16.06.2018_0204_58.zip
md5:4ddc04f88369f7f531ed4efd4d3ad032
19.7 GB Download
204_0p7THz_DyBCO_THG_HWP_130_P2_59_P3_190_P3p5_227_54p7K_16.06.2018_0217_42.zip
md5:56b1a181fc4e1d38e478254e836e1571
19.7 GB Download
205_0p7THz_DyBCO_THG_HWP_134_P2_65_P3_196_P3p5_227_54p7K_16.06.2018_0224_12.zip
md5:afcbd9cfc9bf6c458d769e3fea5a70e7
19.7 GB Download
206_0p7THz_DyBCO_THG_HWP_137_P2_71_P3_202_P3p5_227_54p7K_16.06.2018_0230_38.zip
md5:20f650f456dcc3f2b2f0d16e861e8e32
19.7 GB Download
207_0p7THz_DyBCO_THG_HWP_140_P2_78_P3_209_P3p5_227_54p7K_16.06.2018_0237_02.zip
md5:63e6076e3728987e9b9fb37c4f0dd957
19.7 GB Download
208_0p7THz_DyBCO_THG_HWP_142_P2_82_P3_213_P3p5_227_54p7K_16.06.2018_0243_51.zip
md5:07fb244f0d785b623afa8826fa2ead21
19.7 GB Download
209_0p7THz_DyBCO_THG_HWP_147_P2_94_P3_225_P3p5_227_54p7K_16.06.2018_0250_30.zip
md5:5c79f15c1cc4feae9fcfae3aca4c8e4e
19.8 GB Download
210_0p7THz_DyBCO_THG_HWP_152_P2_106_P3_237_P3p5_227_54p7K_16.06.2018_0258_44.zip
md5:78845224e102cd19ea925267c993b00b
19.8 GB Download
211_0p7THz_DyBCO_THG_HWP_154_P2_110_P3_241_P3p5_227_54p7K_16.06.2018_0305_20.zip
md5:ca7edc2ba1554b1d4df60596b093505f
19.8 GB Download
212_0p7THz_DyBCO_THG_HWP_157_P2_117_P3_248_P3p5_227_54p7K_16.06.2018_0312_22.zip
md5:066d30009183d5a85a4ccb2f4d34322b
19.8 GB Download
213_0p7THz_DyBCO_THG_HWP_160_P2_123_P3_254_P3p5_227_54p7K_16.06.2018_0321_27.zip
md5:b8a9cec48ad5689b3ab408f7fd8ed383
19.1 GB Download
214_0p7THz_DyBCO_THG_HWP_160_P2_123_P3_254_P3p5_227_54p7K_16.06.2018_0411_20.zip
md5:2b096a198793206157dae92bfd07eff9
19.7 GB Download
215_0p7THz_DyBCO_THG_HWP_161_P2_129_P3_260_P3p5_227_54p7K_16.06.2018_0417_37.zip
md5:cafda763f5600cd6571bbf24b2df6e11
19.7 GB Download
216_0p7THz_DyBCO_THG_HWP_161_P2_137_P3_270_P3p5_227_54p7K_16.06.2018_0423_49.zip
md5:af942a5dc8196107101da8beb0c6502a
19.8 GB Download
217_0p7THz_DyBCO_THG_HWP_161_P2_137_P3_270_P3p5_227_54p7K_16.06.2018_0433_51.zip
md5:fc52fe01b7bdfe30f3ae3bedd1ee4416
19.8 GB Download
218_0p7THz_DyBCO_THG_HWP_137_P2_71_P3_202_P3p5_249_54p7K_16.06.2018_0444_37.zip
md5:d6b2de3233bbe6ce922916812613f51f
19.8 GB Download
219_0p7THz_DyBCO_THG_HWP_137_P2_71_P3_112_P3p5_249_54p7K_16.06.2018_0451_27.zip
md5:5adad16c77764f26cc2e4142453d8554
19.8 GB Download
Data analysis.zip
md5:261ddae921a6de6309a506981e89a7d2
1.7 MB Download
Labbook_Dec. 2018 Higgs.zip
md5:10206f47ac188ea12011b5aff7ade675
72.2 MB Download
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40.3 MB Download
README_rodare.txt
md5:98a62a172e5cb650ab5f787fdce4d2e6
2.5 kB Download
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