Dataset Open Access
Rox, Hannes;
Ränke, Fabian;
Zschach, Lis Geraldine;
Yang, Xuegeng;
Mutschke, Gerd;
Eckert, Kerstin;
Lasagni, Andrés Fabián;
Baumann, Robert
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"description": "<p>Tuning the electrode surfaces for better bubble management is a promising approach to increase the efficiency of alkaline water electrolysis. Therefore, Direct Laser Writing was used to structure Nickel electrodes with a dual wetting surface. The applied pillar-like structure combines superhydrophilic behavior and strong spreading of the liquid across the electrode with hydrophobic bubble nucleation sites. In addition, the electrochemically active surface area is increased by a factor of 9. As a result, the overpotential has been significantly reduced, while the size of the detached bubble has increased. The present data set compares three different electrodes, a non-structured reference electrode and two laser structured electrodes with different depths of the structure, at applied current densities of<strong> <em>j</em> = -20, -50 and -100 mA/cm²</strong> in terms of electrode potential, detached bubble size and number of nucleation sites. As electrolyte <strong>1 M KOH</strong> was used. All experiments were carried out under ambient conditions (<strong><em>T</em> = 293 K,<em>p</em> = 1 bar</strong>).</p>\n\n<p><strong>Description of <em>Data.zip</em>:</strong></p>\n\n<p>An overview of all performed experiments is given in the file <strong><em>Summary.csv</em></strong>. The data is analyzed as described in the corresponding journal publication <strong><em>Dual wetting electrode surfaces for alkaline water electrolysis</em></strong>. Each data set is stored in a .hdf5-file, with the relevant metadata incorporated into the attributes assigned to the groups/datasets within the .hdf5-file. The data files are structured in groups as follows:</p>\n\n<ul>\n\t<li>Electrochemical Measurement Data\n\t<ul>\n\t\t<li>Galvanostatic Measurement Data</li>\n\t\t<li>CV double-layer capacitance</li>\n\t\t<li>LSV onset potential</li>\n\t</ul>\n\t</li>\n\t<li>Results\n\t<ul>\n\t\t<li>Detected Bubbles Sideview</li>\n\t</ul>\n\t</li>\n\t<li><em>Sideview Raw Images (only for <strong>SH2_LS_Pil_01.hdf5</strong>)</em></li>\n</ul>\n\n<p>With the exception of a single comprehensive data set comprising unprocessed images (<strong>SH2_LS_Pil_01.hdf5</strong>), the remaining raw images from all performed measurements can be made available upon request.</p>",
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"name": "Rox, Hannes",
"affiliation": "nstitute of Fluid Dynamics, Helmholtz-Zentrum Dresden-Rossendorf, Bautzner Landstrasse 400, Dresden, 01328 Germany",
"orcid": "0000-0003-2826-6903"
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"name": "R\u00e4nke, Fabian",
"affiliation": "Institute of Manufacturing, Technische Universit\u00e4t Dresden, 01062 Dresden, Germany",
"orcid": "0009-0001-4313-9753"
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"name": "Zschach, Lis Geraldine",
"affiliation": "Institute of Manufacturing, Technische Universit\u00e4t Dresden, 01062 Dresden, Germany",
"orcid": "0000-0002-9509-7487"
},
{
"name": "Yang, Xuegeng",
"affiliation": "nstitute of Fluid Dynamics, Helmholtz-Zentrum Dresden-Rossendorf, Bautzner Landstrasse 400, Dresden, 01328 Germany",
"orcid": "0000-0002-4617-0713"
},
{
"name": "Mutschke, Gerd",
"affiliation": "nstitute of Fluid Dynamics, Helmholtz-Zentrum Dresden-Rossendorf, Bautzner Landstrasse 400, Dresden, 01328 Germany",
"orcid": "0000-0002-7918-7474"
},
{
"name": "Eckert, Kerstin",
"affiliation": "nstitute of Fluid Dynamics, Helmholtz-Zentrum Dresden-Rossendorf, Bautzner Landstrasse 400, Dresden, 01328 Germany",
"orcid": "0000-0002-9671-8628"
},
{
"name": "Lasagni, Andr\u00e9s Fabi\u00e1n",
"affiliation": "Institute of Manufacturing, Technische Universit\u00e4t Dresden, 01062 Dresden, Germany",
"orcid": "0000-0003-4333-4636"
},
{
"name": "Baumann, Robert",
"affiliation": "Institute of Manufacturing, Technische Universit\u00e4t Dresden, 01062 Dresden, Germany",
"orcid": "0000-0002-8589-4685"
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"notes": "This project is supported by the Federal State of Saxony in terms of the \"European Regional Development Fund\" (H2-EPF-HZDR), the Helmholtz Association Innovation pool project \"Solar Hydrogen\", the Hydrogen Lab of the School of Engineering of TU Dresden, and BMBF (project ALKALIMIT, grant no. 03SF0731A).",
"title": "Data publication: Dual wetting electrode surfaces for alkaline water electrolysis",
"language": "eng",
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"Alkaline water electrolysis",
"Hydrogen evolution reaction",
"Bubble dynamics",
"Dual wetting",
"Direct laser writing"
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