Fig. 4a: Material/interface dependence of USMR-SHG signal amplitudes. Material / USMR-SHG amplitude / USMR-SHG power Ta2/Py3/Pt2 2.17305E-5 4.72214E-10 Ta2/Co2/Pt2 4.70079E-6 2.20974E-11 Ta3/Py3 3.111E-6 9.67834E-12 Py2/Pt3 9.85521E-6 9.71252E-11 Py2/W3 7.8042E-6 6.09056E-11 Co2/Pt3 2.60045E-6 6.76233E-12 Co2/W3 1.61505E-6 2.60839E-12 Ni2/Pt3 7.19145E-7 5.1717E-13 Ni2/W3 5.39503E-7 2.91063E-13 Time-delay scans of the SHG field for different materials. Delay time / Ta2Py3Pt2 / Ta2Co2Pt2 / Ta3Py3 / Py2Pt3 / Py2W3 / Co2Pt3 / Co2W3 / Ni2Pt3 / Ni2W3 -13.34 1.33962E-5 4.52997E-6 4.7237E-6 -1.4925E-8 1.65404E-5 1.99678E-6 4.7073E-5 3.7551E-6 -2.95043E-6 -13.2066 -1.09971E-5 -7.45075E-7 1.13249E-5 1.1161E-5 5.97542E-6 4.619E-7 1.07139E-5 -1.1772E-6 -9.87948E-6 -13.0732 -2.01316E-5 -1.98185E-6 1.20252E-5 2.04296E-5 -3.72535E-6 5.856E-6 -9.30327E-6 2.06082E-5 -2.03402E-5 -12.9398 -2.3231E-5 -8.15105E-6 9.373E-6 1.95803E-5 -1.05502E-5 -2.101E-6 -1.29144E-5 2.0951E-5 -2.01316E-5 -12.8064 -1.88202E-5 -1.71811E-5 3.66575E-6 1.53184E-5 -1.95206E-5 -1.31283E-5 1.15734E-6 1.51399E-5 -2.16515E-5 -12.673 -2.06382E-5 -2.14876E-5 -1.17718E-6 6.42244E-6 -2.53172E-5 -2.16813E-5 -1.01327E-6 1.2547E-5 -2.56748E-5 -12.5396 -9.65605E-6 -2.95641E-5 -1.04309E-5 -5.06645E-6 -3.06817E-5 -2.55854E-5 1.3734E-5 1.04309E-5 -2.60921E-5 -12.4062 -7.80822E-6 -3.09499E-5 -1.89096E-5 -1.63318E-5 -3.47795E-5 -2.86104E-5 2.15671E-5 9.8944E-6 -2.60922E-5 -12.2728 -3.8295E-6 -3.52565E-5 -1.76132E-5 -2.83421E-5 -3.53458E-5 -2.49448E-5 2.25158E-5 8.00202E-6 -2.51384E-5 -12.1394 4.475E-8 -3.25144E-5 -2.19047E-5 -3.30211E-5 -3.6359E-5 -2.10853E-5 2.27742E-5 -3.81467E-6 -2.44676E-5 -12.006 7.51E-6 -2.75824E-5 -2.04598E-5 -3.52118E-5 -3.16801E-5 -1.19955E-5 2.38369E-5 -1.06547E-5 -1.42305E-5 -11.8726 1.42455E-5 -2.41105E-5 -1.51395E-5 -3.21723E-5 -2.38867E-5 -5.75175E-6 1.7792E-5 -1.66592E-5 -2.9055E-6 -11.7392 2.16817E-5 -1.92376E-5 -1.12355E-5 -2.86848E-5 -1.66892E-5 -3.77E-6 1.51147E-5 -2.4378E-5 1.24572E-5 -11.6058 2.51835E-5 -1.12357E-5 -6.1245E-6 -2.25752E-5 -1.40219E-5 -4.77E-7 1.69677E-5 -3.00703E-5 2.29927E-5 -11.4724 2.78205E-5 -6.28827E-6 -3.54675E-6 -1.28598E-5 -1.26512E-5 1.29625E-6 1.45188E-5 -2.83867E-5 3.29466E-5 -11.339 3.15162E-5 -2.48858E-6 -4.2468E-6 -1.15187E-5 -3.82965E-6 2.54775E-6 1.43003E-5 -2.5943E-5 3.39749E-5 -11.2056 2.17856E-5 2.51822E-6 -4.18723E-6 -9.4921E-6 6.00521E-6 -4.6225E-7 8.54333E-6 -2.91026E-5 3.39152E-5 -11.0722 1.91034E-5 7.39104E-6 -6.13933E-6 -4.30646E-6 1.47373E-5 9.53675E-7 4.41078E-6 -3.02047E-5 3.32298E-5 -10.9388 1.18316E-5 1.55868E-5 -9.07483E-6 3.30805E-6 2.63752E-5 4.39585E-6 1.02324E-6 -2.64945E-5 3.41536E-5 -10.8054 5.15583E-6 2.08766E-5 -6.25835E-7 8.50853E-6 3.3185E-5 3.03983E-6 -3.91404E-6 -1.7047E-5 3.19631E-5 -10.672 -1.04303E-6 2.4766E-5 7.62945E-6 1.92824E-5 3.66124E-5 7.67413E-6 -7.83813E-6 -1.1623E-6 3.05178E-5 -10.5386 -5.2749E-6 2.67924E-5 7.42077E-6 2.50938E-5 3.84601E-5 1.09524E-5 -8.02182E-6 7.689E-6 2.83422E-5 -10.4052 -9.03025E-6 3.04729E-5 1.1608E-5 3.22162E-5 3.59418E-5 1.23826E-5 -1.12007E-5 9.38755E-6 2.30074E-5 -10.2718 -9.299E-6 2.82975E-5 1.0729E-5 3.64631E-5 3.12628E-5 1.01327E-5 -1.52193E-5 1.76433E-5 1.77474E-5 -10.1384 -1.01335E-5 2.18899E-5 1.05945E-5 3.79832E-5 2.17855E-5 7.54E-6 -1.62725E-5 2.41848E-5 5.0068E-6 -10.005 -1.12354E-5 1.47671E-5 1.1295E-5 3.40492E-5 1.43946E-5 5.48375E-6 -1.46229E-5 2.55107E-5 -8.49367E-6 -9.8716 -1.27554E-5 5.17073E-6 1.3456E-5 2.56301E-5 5.91585E-6 2.548E-6 -9.61128E-6 2.34105E-5 -2.59134E-5 -9.7382 -1.36943E-5 1.6093E-6 1.20998E-5 1.62274E-5 1.87753E-6 3.77025E-6 -8.24542E-6 2.3872E-5 -2.94448E-5 -9.6048 -1.87905E-5 -1.90737E-6 4.55975E-6 7.73374E-6 -4.14254E-6 1.53428E-6 -6.49193E-6 2.30224E-5 -3.72829E-5 -9.4714 -1.82987E-5 -7.52518E-6 -6.94398E-6 2.57787E-6 -1.28002E-5 -4.35118E-6 -8.24535E-6 2.66285E-5 -4.19619E-5 -9.338 -1.75835E-5 -1.07139E-5 -1.30535E-5 -7.40585E-6 -1.70768E-5 -9.56663E-6 -8.82648E-6 2.2188E-5 -4.22153E-5 -9.2046 -1.29939E-5 -1.72109E-5 -1.7509E-5 -1.32323E-5 -2.40954E-5 -1.19359E-5 -1.36496E-5 1.61231E-5 -4.15893E-5 -9.0712 -7.10785E-6 -2.41847E-5 -1.5229E-5 -2.28287E-5 -2.86251E-5 -1.02967E-5 -6.08942E-6 1.02968E-5 -3.94732E-5 -8.9378 -5.365E-7 -2.59131E-5 -1.67192E-5 -2.91765E-5 -2.78203E-5 -8.61285E-6 -2.50342E-6 5.28995E-6 -3.88627E-5 -8.8044 6.259E-6 -2.77459E-5 -1.5989E-5 -3.51071E-5 -2.60472E-5 -7.3613E-6 1.28658E-6 -4.6939E-6 -3.21422E-5 -8.671 1.3948E-5 -2.39762E-5 -1.84478E-5 -3.83406E-5 -2.26795E-5 -9.70075E-6 5.46867E-6 -1.11462E-5 -2.62113E-5 -8.5376 1.9178E-5 -1.66001E-5 -1.51845E-5 -3.97711E-5 -2.0087E-5 -8.5235E-6 6.527E-6 -1.74645E-5 -1.50802E-5 -8.4042 2.27398E-5 -8.53843E-6 -1.4514E-5 -3.31849E-5 -1.91033E-5 -7.659E-6 5.33983E-6 -1.90145E-5 -6.6906E-6 -8.2708 2.78951E-5 -7.43568E-6 -1.7271E-5 -2.41699E-5 -1.96251E-5 -2.667E-6 -1.29644E-6 -2.17115E-5 1.15336E-5 -8.1374 2.89531E-5 -4.96215E-6 -1.90137E-5 -1.85967E-5 -1.88948E-5 1.654E-6 -1.10964E-5 -2.04595E-5 1.98485E-5 -8.004 3.03241E-5 -6.51186E-6 -2.05638E-5 -1.05799E-5 -1.08183E-5 9.2095E-6 -1.41463E-5 -2.04593E-5 2.59878E-5 -7.8706 2.26052E-5 -7.67411E-6 -1.56313E-5 -3.75513E-6 -5.15577E-6 1.30981E-5 -1.02173E-5 -2.25754E-5 3.26188E-5 -7.7372 1.16379E-5 -1.9222E-6 -9.25367E-6 -9.834E-7 4.73867E-6 9.56653E-6 -3.36272E-6 -2.21581E-5 3.40046E-5 -7.6038 6.70475E-7 3.51667E-6 -1.41558E-6 6.4075E-7 1.57505E-5 6.03501E-6 5.92571E-6 -2.13088E-5 3.49732E-5 -7.4704 -6.06483E-6 1.41563E-5 2.35432E-6 4.3212E-6 2.54066E-5 7.58468E-6 5.9358E-6 -1.46032E-5 3.58378E-5 -7.337 -1.38585E-5 1.8254E-5 7.43565E-6 1.22043E-5 3.40198E-5 5.57303E-6 4.92767E-6 -9.79013E-6 3.6374E-5 -7.2036 -1.24575E-5 2.13685E-5 1.09225E-5 2.11155E-5 3.33195E-5 7.6E-6 1.11775E-6 -2.66752E-6 3.3111E-5 -7.0702 -1.33068E-5 1.90445E-5 1.13397E-5 2.85363E-5 2.95937E-5 7.0335E-6 7.4025E-7 6.00525E-6 2.68225E-5 -6.9368 -7.88275E-6 1.7763E-5 1.22045E-5 3.15757E-5 2.31565E-5 9.3875E-6 3.075E-7 1.07435E-5 1.68985E-5 -6.8034 -5.3345E-6 1.87011E-5 1.41112E-5 3.57036E-5 1.59589E-5 1.05203E-5 -7.99417E-7 1.5885E-5 8.9555E-6 -6.67 -2.7715E-6 1.54525E-5 1.38137E-5 3.86238E-5 9.31323E-6 9.35775E-6 2.6835E-7 2.1428E-5 -8.34525E-7 -6.5366 -3.87175E-7 1.39475E-5 1.7405E-5 3.53905E-5 3.75505E-6 5.5135E-6 -2.50337E-6 2.25007E-5 -1.02372E-5 -6.4032 1.7285E-6 9.65597E-6 1.63318E-5 3.06519E-5 -1.7732E-6 -2.56275E-6 -3.33792E-6 2.15325E-5 -1.78369E-5 -6.2698 -2.57795E-6 2.8611E-6 1.60934E-5 2.63603E-5 -6.52674E-6 -7.853E-6 -2.65244E-6 2.19198E-5 -2.87594E-5 -6.1364 -1.90738E-6 -4.24683E-6 1.14441E-5 1.49907E-5 -1.13249E-5 -1.70764E-5 -6.41749E-6 1.94311E-5 -3.25145E-5 -6.003 -7.61452E-6 -1.13696E-5 5.0813E-6 1.89246E-6 -1.61083E-5 -1.75536E-5 -5.22039E-6 1.85969E-5 -3.26934E-5 -5.8696 -1.1012E-5 -1.78219E-5 9.23878E-7 -1.29343E-5 -1.67491E-5 -1.63764E-5 -6.80994E-6 1.71662E-5 -3.32744E-5 -5.7362 -1.51396E-5 -2.20688E-5 -8.34465E-7 -2.26797E-5 -1.81347E-5 -1.44989E-5 -7.15754E-6 1.1757E-5 -3.41239E-5 -5.6028 -1.18763E-5 -2.44678E-5 -9.84972E-6 -3.168E-5 -1.49608E-5 -9.73051E-6 -2.58783E-6 8.46388E-6 -2.9892E-5 -5.4694 -6.30317E-6 -2.42444E-5 -1.36495E-5 -3.70593E-5 -1.54377E-5 -5.40915E-6 -1.97687E-6 6.184E-6 -2.67925E-5 -5.336 8.44918E-6 -2.17112E-5 -1.53037E-5 -4.19023E-5 -1.67192E-5 -4.0979E-6 -3.52662E-6 -1.23677E-6 -2.09512E-5 -5.2026 1.9327E-5 -1.72706E-5 -1.62872E-5 -4.26175E-5 -1.76729E-5 -3.74023E-6 2.38425E-7 -7.25695E-6 -1.50502E-5 -5.0692 3.01006E-5 -1.31428E-5 -1.70919E-5 -3.89965E-5 -1.71513E-5 -3.48687E-6 4.91738E-6 -1.6913E-5 -1.04457E-5 -4.9358 3.76555E-5 -1.22488E-5 -1.58402E-5 -3.0935E-5 -1.70321E-5 -7.06313E-6 6.42734E-6 -2.11747E-5 -2.54812E-6 -4.8024 3.92201E-5 -1.11015E-5 -1.17422E-5 -2.19644E-5 -1.31578E-5 -6.0051E-6 4.56475E-6 -2.18601E-5 5.69226E-6 -4.669 3.4705E-5 -5.26018E-6 -6.78003E-6 -1.57506E-5 -1.08928E-5 -1.62428E-6 4.29157E-6 -2.28586E-5 1.28598E-5 -4.5356 1.70023E-5 -3.03986E-6 -3.84448E-6 -9.6262E-6 -3.4422E-6 5.79655E-6 2.55805E-6 -1.89545E-5 1.94908E-5 -4.4022 -2.57792E-6 5.5135E-7 1.49E-7 -6.89929E-6 2.48852E-6 1.12654E-5 1.68383E-6 -1.70769E-5 2.50937E-5 -4.2688 -1.71662E-5 1.87758E-6 1.89247E-6 -5.37932E-6 9.1642E-6 1.45585E-5 3.17888E-6 -1.15782E-5 2.943E-5 -4.1354 -3.15608E-5 3.74015E-6 3.14417E-6 -1.80303E-6 1.32472E-5 1.6004E-5 9.76524E-6 -8.82153E-6 3.07563E-5 -4.002 -3.84154E-5 2.22028E-6 4.73861E-6 4.11272E-6 1.99825E-5 1.68831E-5 1.49906E-5 -4.21702E-6 3.18292E-5 -3.8686 -3.46901E-5 1.92225E-6 2.96533E-6 1.02222E-5 2.17409E-5 1.72407E-5 1.74691E-5 -2.96535E-6 3.17099E-5 -3.7352 -2.48851E-5 7.59925E-7 4.0978E-6 1.98187E-5 2.58686E-5 1.37837E-5 1.55718E-5 2.16069E-6 2.7761E-5 -3.6018 -1.1012E-5 5.91575E-6 5.93067E-6 3.16801E-5 2.89084E-5 1.359E-5 8.94568E-6 7.12277E-6 2.2337E-5 -3.4684 9.73052E-6 1.02819E-5 4.99191E-6 4.51806E-5 2.99068E-5 1.06245E-5 1.42554E-6 1.28747E-5 1.50056E-5 -3.335 2.04892E-5 1.31876E-5 4.45548E-6 5.32719E-5 1.93269E-5 9.2238E-6 -5.20546E-6 1.42605E-5 1.14292E-5 -3.2016 3.46305E-5 1.30386E-5 7.70392E-6 5.54476E-5 9.99877E-6 9.4772E-6 -9.57153E-6 1.74047E-5 2.02658E-6 -3.0682 3.28423E-5 1.61977E-5 1.18316E-5 5.35698E-5 7.51015E-6 9.43253E-6 -1.26363E-5 2.16813E-5 -2.414E-6 -2.9348 2.08172E-5 1.29193E-5 9.40275E-6 4.55381E-5 2.05675E-6 6.34793E-6 -1.16825E-5 2.48851E-5 -1.47819E-5 -2.8014 5.84123E-6 6.18427E-6 6.95885E-6 3.04582E-5 -4.81325E-6 1.6094E-6 -9.16467E-6 2.31415E-5 -2.18005E-5 -2.668 -1.24871E-5 1.2215E-6 7.853E-6 1.19807E-5 -5.11125E-6 -4.0382E-6 -8.71733E-6 1.74345E-5 -2.61965E-5 -2.5346 -2.44528E-5 -4.903E-6 7.40592E-6 -3.18895E-6 -4.79825E-6 -9.44748E-6 -9.41733E-6 1.35007E-5 -2.46168E-5 -2.4012 -2.70159E-5 -5.55802E-6 3.621E-6 -1.56313E-5 2.63725E-6 -1.44395E-5 -1.31431E-5 8.07663E-6 -2.45428E-5 -2.2678 -2.2948E-5 -9.86452E-6 3.24842E-6 -2.67477E-5 1.80306E-5 -2.02658E-5 -1.31331E-5 1.08785E-6 -2.79551E-5 -2.1344 -1.1906E-5 -9.19412E-6 8.6425E-7 -2.96088E-5 1.65404E-5 -2.41699E-5 -1.71861E-5 -2.02658E-6 -2.55855E-5 -2.001 2.80144E-6 -3.30801E-6 -1.27256E-5 -3.62995E-5 1.48268E-5 -2.72991E-5 -1.25915E-5 -5.72205E-6 -2.68819E-5 -1.8676 2.7001E-5 -1.17719E-6 -1.18316E-5 -3.26486E-5 5.6625E-6 -2.52129E-5 -7.31649E-6 -1.21892E-5 -2.13982E-5 -1.7342 4.60001E-5 4.0235E-7 -1.84477E-5 -2.60326E-5 -7.71882E-6 -1.87309E-5 -8.48374E-6 -1.75983E-5 -2.81783E-5 -1.6008 5.75635E-5 5.27495E-6 -1.96995E-5 -2.06679E-5 -2.22327E-5 -1.00435E-5 -9.06977E-6 -1.78964E-5 -1.46926E-5 -1.4674 5.5149E-5 1.42604E-5 -1.65105E-5 -1.31726E-5 -3.04139E-5 -5.11118E-6 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