Fig. 3ab: SHG intensity in the Ta(2nm)/Py(3nm)/Pt(2nm) sample as a function of the THz pump polarisation angle, measured in a vertical and horizontal magnetisation geometry. Calculated Measured THz polarization angle / SHG intensity for Horizontal magetization / SHG intensity for Vertical magetization 0.5 3.42312E-15 1.15193E-10 0 1.18338E-12 9.32044E-11 1 1.36883E-14 1.15174E-10 15 5.41566E-12 1.14388E-10 1.5 3.07831E-14 1.15141E-10 30 9.77208E-12 9.98525E-11 2 5.46867E-14 1.15095E-10 45 1.19691E-11 8.00733E-11 2.5 8.537E-14 1.15036E-10 60 7.34971E-12 5.29388E-11 3 1.22796E-13 1.14964E-10 75 3.49346E-12 4.12664E-11 3.5 1.66918E-13 1.14879E-10 90 4.56205E-13 3.585E-11 4 2.17684E-13 1.1478E-10 4.5 2.7503E-13 1.14669E-10 5 3.38889E-13 1.14545E-10 5.5 4.09181E-13 1.14408E-10 6 4.85821E-13 1.14259E-10 6.5 5.68716E-13 1.14097E-10 7 6.57766E-13 1.13922E-10 7.5 7.52861E-13 1.13734E-10 8 8.53886E-13 1.13534E-10 8.5 9.60718E-13 1.13322E-10 9 1.07323E-12 1.13097E-10 9.5 1.19128E-12 1.12861E-10 10 1.31472E-12 1.12612E-10 10.5 1.44341E-12 1.12351E-10 11 1.57719E-12 1.12079E-10 11.5 1.7159E-12 1.11795E-10 12 1.85937E-12 1.11499E-10 12.5 2.00741E-12 1.11192E-10 13 2.15987E-12 1.10874E-10 13.5 2.31653E-12 1.10544E-10 14 2.47723E-12 1.10204E-10 14.5 2.64176E-12 1.09852E-10 15 2.80991E-12 1.09491E-10 15.5 2.9815E-12 1.09118E-10 16 3.1563E-12 1.08735E-10 16.5 3.33411E-12 1.08343E-10 17 3.5147E-12 1.0794E-10 17.5 3.69786E-12 1.07527E-10 18 3.88337E-12 1.07105E-10 18.5 4.071E-12 1.06673E-10 19 4.26052E-12 1.06233E-10 19.5 4.4517E-12 1.05783E-10 20 4.64431E-12 1.05324E-10 20.5 4.83811E-12 1.04857E-10 21 5.03287E-12 1.04381E-10 21.5 5.22835E-12 1.03897E-10 22 5.42431E-12 1.03406E-10 22.5 5.62052E-12 1.02906E-10 23 5.81673E-12 1.02399E-10 23.5 6.01271E-12 1.01884E-10 24 6.20822E-12 1.01363E-10 24.5 6.40302E-12 1.00834E-10 25 6.59687E-12 1.00299E-10 25.5 6.78954E-12 9.97572E-11 26 6.98079E-12 9.92094E-11 26.5 7.17039E-12 9.86555E-11 27 7.35811E-12 9.80959E-11 27.5 7.54372E-12 9.75308E-11 28 7.72699E-12 9.69604E-11 28.5 7.90771E-12 9.63849E-11 29 8.08565E-12 9.58046E-11 29.5 8.26059E-12 9.52197E-11 30 8.43233E-12 9.46305E-11 30.5 8.60064E-12 9.40372E-11 31 8.76534E-12 9.34399E-11 31.5 8.92622E-12 9.28391E-11 32 9.08307E-12 9.22348E-11 32.5 9.23572E-12 9.16273E-11 33 9.38397E-12 9.10169E-11 33.5 9.52765E-12 9.04039E-11 34 9.66658E-12 8.97883E-11 34.5 9.80059E-12 8.91705E-11 35 9.92952E-12 8.85507E-11 35.5 1.00532E-11 8.79291E-11 36 1.01715E-11 8.7306E-11 36.5 1.02843E-11 8.66816E-11 37 1.03914E-11 8.60561E-11 37.5 1.04927E-11 8.54297E-11 38 1.0588E-11 8.48027E-11 38.5 1.06774E-11 8.41752E-11 39 1.07605E-11 8.35476E-11 39.5 1.08375E-11 8.292E-11 40 1.0908E-11 8.22926E-11 40.5 1.09722E-11 8.16657E-11 41 1.10298E-11 8.10395E-11 41.5 1.10809E-11 8.04141E-11 42 1.11253E-11 7.97898E-11 42.5 1.11631E-11 7.91668E-11 43 1.11941E-11 7.85452E-11 43.5 1.12183E-11 7.79254E-11 44 1.12357E-11 7.73074E-11 44.5 1.12463E-11 7.66916E-11 45 1.125E-11 7.6078E-11 45.5 1.12469E-11 7.54668E-11 46 1.12369E-11 7.48583E-11 46.5 1.12201E-11 7.42526E-11 47 1.11966E-11 7.36499E-11 47.5 1.11662E-11 7.30504E-11 48 1.11291E-11 7.24542E-11 48.5 1.10852E-11 7.18616E-11 49 1.10348E-11 7.12726E-11 49.5 1.09777E-11 7.06875E-11 50 1.09142E-11 7.01064E-11 50.5 1.08442E-11 6.95295E-11 51 1.07678E-11 6.89569E-11 51.5 1.06852E-11 6.83887E-11 52 1.05964E-11 6.78252E-11 52.5 1.05016E-11 6.72664E-11 53 1.04009E-11 6.67125E-11 53.5 1.02943E-11 6.61636E-11 54 1.0182E-11 6.56199E-11 54.5 1.00642E-11 6.50814E-11 55 9.94103E-12 6.45484E-11 55.5 9.81257E-12 6.40209E-11 56 9.67902E-12 6.34991E-11 56.5 9.54054E-12 6.29831E-11 57 9.39728E-12 6.24729E-11 57.5 9.24944E-12 6.19687E-11 58 9.09719E-12 6.14706E-11 58.5 8.94071E-12 6.09787E-11 59 8.78019E-12 6.0493E-11 59.5 8.61583E-12 6.00138E-11 60 8.44784E-12 5.95411E-11 60.5 8.27641E-12 5.90749E-11 61 8.10175E-12 5.86153E-11 61.5 7.92407E-12 5.81626E-11 62 7.7436E-12 5.77166E-11 62.5 7.56055E-12 5.72775E-11 63 7.37514E-12 5.68454E-11 63.5 7.18761E-12 5.64203E-11 64 6.99817E-12 5.60023E-11 64.5 6.80706E-12 5.55915E-11 65 6.61451E-12 5.51879E-11 65.5 6.42076E-12 5.47916E-11 66 6.22604E-12 5.44026E-11 66.5 6.03059E-12 5.40211E-11 67 5.83464E-12 5.3647E-11 67.5 5.63844E-12 5.32804E-11 68 5.44222E-12 5.29213E-11 68.5 5.24622E-12 5.25699E-11 69 5.05069E-12 5.22261E-11 69.5 4.85586E-12 5.18899E-11 70 4.66196E-12 5.15615E-11 70.5 4.46923E-12 5.12408E-11 71 4.27791E-12 5.09279E-11 71.5 4.08823E-12 5.06229E-11 72 3.90042E-12 5.03257E-11 72.5 3.71471E-12 5.00363E-11 73 3.53132E-12 4.97549E-11 73.5 3.35048E-12 4.94814E-11 74 3.17241E-12 4.92158E-11 74.5 2.99733E-12 4.89582E-11 75 2.82544E-12 4.87087E-11 75.5 2.65696E-12 4.84671E-11 76 2.49209E-12 4.82336E-11 76.5 2.33104E-12 4.80081E-11 77 2.174E-12 4.77907E-11 77.5 2.02115E-12 4.75814E-11 78 1.87269E-12 4.73801E-11 78.5 1.7288E-12 4.7187E-11 79 1.58965E-12 4.7002E-11 79.5 1.45542E-12 4.68251E-11 80 1.32625E-12 4.66564E-11 80.5 1.20232E-12 4.64958E-11 81 1.08378E-12 4.63433E-11 81.5 9.70756E-13 4.61991E-11 82 8.634E-13 4.6063E-11 82.5 7.6184E-13 4.5935E-11 83 6.66199E-13 4.58153E-11 83.5 5.76593E-13 4.57037E-11 84 4.93131E-13 4.56004E-11 84.5 4.15916E-13 4.55052E-11 85 3.45041E-13 4.54182E-11 85.5 2.80592E-13 4.53395E-11 86 2.22647E-13 4.52689E-11 86.5 1.71278E-13 4.52066E-11 87 1.26547E-13 4.51524E-11 87.5 8.85078E-14 4.51065E-11 88 5.72073E-14 4.50688E-11 88.5 3.26834E-14 4.50393E-11 89 1.4966E-14 4.5018E-11 89.5 4.07663E-15 4.50049E-11 90 2.85361E-17 4.5E-11